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Collision photography: polarization imaging of atom-molecule collisions

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Authors

Goldstein, R.
Figl, C.
Grosser, J.
Hoffmann, O.
Jungen, M.
Stalder, J.
Rebentrost, F.

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American Institute of Physics (AIP)

Abstract

We report differential scattering experiments on the laser excitation of Na+Mcollision pairs with M=N₂, CO, C₂H₂, and CO₂. The collision event is probed by the laser polarization revealing geometric and electronic properties of the collision pair. The experimental data are compared to the results of a Monte Carlo trajectory simulation using ab initio quantum chemical data.

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The Journal of Chemical Physics

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