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What does the Sr-substituted 2.1 Å resolution crystal structure of photosystem II reveal about the water oxidation mechanism?

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dc.contributor.authorTerrett, Richard
dc.contributor.authorPetrie, Simon
dc.contributor.authorPace, Ronald
dc.contributor.authorStranger, Robert
dc.date.accessioned2015-12-10T23:07:34Z
dc.date.issued2014
dc.date.updated2015-12-10T09:00:18Z
dc.description.abstractA density functional study of the Sr-substituted photosystem II water oxidising complex demonstrates that its recent X-ray crystal structure is consistent with a (MnIII)4 oxidation state pattern, and with a Sr-bound hydroxide ion. The Sr-water-hydroxide interactions rationalize differences in the exchange rates of substrate water and kinetics of dioxygen bond formation relative to the Ca-containing structure.
dc.identifier.issn1359-7345
dc.identifier.urihttp://hdl.handle.net/1885/62936
dc.publisherRoyal Society of Chemistry
dc.sourceChemical Communications
dc.titleWhat does the Sr-substituted 2.1 Å resolution crystal structure of photosystem II reveal about the water oxidation mechanism?
dc.typeJournal article
local.bibliographicCitation.issue24
local.bibliographicCitation.lastpage3190
local.bibliographicCitation.startpage3187
local.contributor.affiliationTerrett, Richard, College of Physical and Mathematical Sciences, ANU
local.contributor.affiliationPetrie, Simon, College of Physical and Mathematical Sciences, ANU
local.contributor.affiliationPace, Ronald, College of Physical and Mathematical Sciences, ANU
local.contributor.affiliationStranger, Robert, College of Physical and Mathematical Sciences, ANU
local.contributor.authoruidTerrett, Richard, u4125581
local.contributor.authoruidPetrie, Simon, u9800071
local.contributor.authoruidPace, Ronald, u8202121
local.contributor.authoruidStranger, Robert, u8708796
local.description.embargo2037-12-31
local.description.notesImported from ARIES
local.identifier.absfor030701 - Quantum Chemistry
local.identifier.absseo970103 - Expanding Knowledge in the Chemical Sciences
local.identifier.ariespublicationu4005981xPUB752
local.identifier.citationvolume50
local.identifier.doi10.1039/c3cc49324e
local.identifier.scopusID2-s2.0-84896840729
local.identifier.thomsonID000332115400015
local.type.statusPublished Version

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